Dynamics of heterogeneous clusters under intense X-ray pulses

Pierfrancesco Di Cintio

MPI für Physik komplexer Systeme, Dresden, Germany

We study the interaction of short and intense X-ray pulses with clusters of protonated molecules such as CH4 and H2O, [1]. We find that due to the effective positive charge outflow (i.e. faster expansion of the proton component see e.g. [2] and references therein) that lowers the cluster potential formed by the massive ionization, the temperature of the electron plasma generated inside the cluster is sensibly lower than in the case of a pure atomic cluster where no positive charge loss is possible. We argue that the relatively low electron temperature is responsible for the effcient recombination of the electrons on molecular fragments recently observed in experiments at LCLS [3].

References
[1] Di Cintio P.F., Gnodtke C., Saalmann U. and Rost J.M. \Dynamics of methane clusters under short XFEL pulses", 2012, in preparation.
[2] Popov K.I., Bychenkov V. Y., Rozmus W., Kovalev V.F. and Sydora R.D., \Mono-energetic ions from collisionless expansion of spherical multi-species clusters", 2009, Laser and Particle Beams 27, 321.
[3] Kandadai, N. et al., 2012, in preparation.

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